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"Long-lasting, reinforced electrical networking in a high-loading Li2S " by Hun Kim, Kyeong Jun Min et al.

Realizing a lithium sulfide (Li2S) cathode with both high energy density and a long lifespan requires an innovative cathode design that maximizes electrochemical performance and resists electrode deterioration. Herein, a high-loading Li2S-based cathode with micrometric Li2S particles composed of two-dimensional graphene (Gr) and one-dimensional carbon nanotubes (CNTs) in a compact geometry is developed, and the role of CNTs in stable cycling of high-capacity Li–S batteries is emphasized. In a dimensionally combined carbon matrix, CNTs embedded within the Gr sheets create robust and sustainable electron diffusion pathways while suppressing the passivation of the active carbon surface. As a unique point, during the first charging process, the proposed cathode is fully activated through the direct conversion of Li2S into S8 without inducing lithium polysulfide formation. The direct conversion of Li2S into S8 in the composite cathode is ubiquitously investigated using the combined study ....

Carbon Nanotubes , Electrical Network , High Energy , High Loading , Is Cathode 2 , Lithium Sulfur Batteries ,