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"Creating New MOF-based Interfaces for Electrocatalytic CO2 Reduction" by Lisha Jia

Metal-organic frameworks (MOFs)-based materials is a promising candidate as electrolycatalysts for energy conversion. MOF-derived materials have been widely employed as catalysts for overall water splitting, benefiting from MOF precursors’ unique porous structure, large surface area, and adjustable morphology/thickness, etc. Also, MOFs work well as desirable catalysts for mainly CO and formate production in electrochemical CO2 reduction reaction (CO2RR). Cu-based MOFs acting as catalysts have demonstrated great potential for producing formate. In this thesis, one MOF-derived catalyst and two MOFs catalysts were designed and prepared for water splitting and CO2RR. The thesis provided strategies to boost conductivity, hence stability, and decrease the agglomeration of MOF-based catalysts and investigated the effect of electrolyte solvent on CO2RR. ....

Overall Water Splitting ,

Study suggests energy-efficient route to capturing and converting CO2

MIT researchers found how carbon dioxide can be captured and converted through a single electrochemical process. A system based on these findings could help cut emissions from the hardest-to-decarbonize industries, such as steel and cement. ....

Aisyah Illyani Ismail , Elizabeth Bernhardt , Arif Arifutzzaman , Graham Leverick , Mohamed Kheireddine Aroua , Sunway University , Career Development Associate Professor , Betar Gallant , Development Associate Professor , Jun Hui Law , Mit Meche , Betar Gallant , Graham Leverick , Carbon Storage , Carbon Conversion , Industrial Decarbonization ,