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Abstract
The fabrication of highly durable, flexible, all-solid-state supercapacitors (ASCs) remains challenging because of the unavoidable mechanical stress that such devices are subjected to in wearable applications. Natural/artificial fiber textiles are regarded as prospective materials for flexible ASCs due to their outstanding physicochemical properties. Here, a high-performance ASC is designed by employing graphene-encapsulated polyester fiber loaded with polyaniline as the flexible electrodes and bacterial cellulose (BC) nanofiber-reinforced polyacrylamide as the hydrogel electrolyte. The ASC combines the textile electrode capable of arbitrary deformation with the BC-reinforced hydrogel with high ionic conductivity (125 mS cm ), high tensile strength (330 kPa), and superelasticity (stretchability up to ≈1300%), giving rise to a device with high stability/compatibility between the electrodes and electrolyte that is compliant with flexible electronics. As a result, this ASC d